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Water Water Everywhere Hydrogen’s Nowhere to Be Seen: But Get Some Catalyst Cheap But Right Enough and May You Make Cheap and Easy Hydrogen to Be Clean and Green: New Research Makes Way Into Breaking Hydrogen Free From Water

 

 

 

 

 

 

 

 

 

 

 

 

 

 

 

 

 

 

|| January 27: 2019: University of Glasgow News || ά. An international collaboration between researchers in Spain and Scotland has resulted in a new approach to improve the catalysts needed to carry out the Hydrogen Evolution Reaction:HER. The reaction, in which, water is transformed into hydrogen and oxygen, is a promising alternative to humanity’s dependency on fossil fuels to satisfy energy requirements.

The research results, published in Nature Communications, demonstrate that molecular HER-catalysts can work in an efficient manner while highlighting the fundamental importance of understanding the underlying catalyst-water interactions and the fine balance of numerous parameters, affecting the evolution of hydrogen. Mr Carles Bo, the Group Leader at the Institute of Chemical Research of Catalonia:ICIQ, is one of the lead authors on the paper. He said, “We are trying to find catalysts cheaper than the noble-metal based ones used right now, to make economically viable the production of hydrogen from water. These findings will accelerate the development of a hydrogen-based economy.”

The combination of theoretical and experimental approaches has allowed the scientists to gain some mechanistic insights into the Hydrogen Evolution Reaction and to explore how the new catalysts work.  Dr Haralampos Miras, Senior Lecturer at the University of Glasgow's School of Chemistry, said, “We are interested in making molecules, designed to tackle challenging tasks, such as, the evolution of hydrogen from water and understand how these molecules work.”

MoS2 is a promising material for the electro-catalytic generation of hydrogen from water. However, tuning the two-D material for an efficient catalyst-water interaction is no trivial matter. Here, the scientists have used MoS2 as a starting point to design molecular analogues, that mimic its catalytically active sites while exposing a high number of them.

The family of molecular catalysts described in the paper were designed, using modular approaches, that ensure an efficient interaction between the catalytic sites and the water molecules, while avoiding expensive noble metals. The fact that the new catalysts’ synthesis is carried out open to air and in a simple two-step process, hints at the potential of the approaches for scalability and its economic viability to compete with advanced platinum-based catalysts.

The result of the EU funded COST Action Polyoxometalate Chemistry for Molecular Nanoscience, the scientists have worked together for several years to develop the approach presented in the paper.

Dr Miras said, “It becomes apparent, even, to the most sceptical members of public and political figures that the depleting fossil fuels reserves and the unprecedented environmental consequences that we are, already, experiencing, require urgent and decisive actions. Our work is part of a worldwide effort towards a hydrogen-based economy. We anticipate these findings to be a starting point for further exploration of molecular catalytic systems and inspire others in an effort to tackle challenging scientific issues." :::ω.

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New Research Discovers New Quantum Spin Liquid

 

 

|| January 23: 2019: University of Liverpool News || ά. An international research team, led by the University of Liverpool and McMaster University has made a significant breakthrough in the search for new states of matter. In a study, published in the journal Nature Physics, researchers show that the perovskite-related metal oxide, TbInO3, exhibits a quantum spin liquid state, a long-sought-after and unusual state of matter. Using advanced experimental technologies, including, inelastic neutron scattering and muon spectroscopy, researchers discovered that the exotic quantum state in TbInO3 emerges from the complexity of the local environment around the magnetic ions in the material, in this case, of the rare-earth element terbium.

The discovery came as a surprise to the team as TbInO3 is a material not expected to display such unusual magnetic behaviour, based on its crystal structure. The quantum spin liquid state was theoretically proposed over forty years ago by the Nobel laureate Philip Anderson. In quantum spin liquids, magnetic moments behave like a liquid and do not freeze or order, even, at absolute zero, giving rise to several extraordinary materials properties. The materialisation of quantum spin liquids is still widely contested. As such, the discovery and exploration of new materials, that, may, host this state of matter are active areas of advanced materials research and have potential applications in the development of quantum computing.

Dr Lucy Clark, from the University’s